Anode optimization strategies for aqueous zinc-ion batteries

Publication Name

Chemical Science

Abstract

Zinc-ion batteries (ZIBs) have received much research attention due to their advantages of safety, non-toxicity, simple manufacture, and element abundance. Nevertheless, serious problems still remain for their anodes, such as dendrite development, corrosion, passivation, and the parasitic hydrogen evolution reaction due to their unique aqueous electrolyte system constituting the main issues that must be addressed, which are blocking the further advancement of anodes for Zn-ion batteries. Herein, we conduct an in-depth analysis of the problems that exist for the zinc anode, summarize the main failure types and mechanisms of the zinc anode, and review the main modification strategies for the anode from the three aspects of the electrolyte, anode surface, and anode host. Furthermore, we also shed light on further modification and optimization strategies for the zinc anode, which provide directions for the future development of anodes for zinc-ion batteries.

Open Access Status

This publication may be available as open access

Volume

13

Issue

48

First Page

14246

Last Page

14263

Funding Number

2021C04019

Funding Sponsor

Australian Research Council

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Link to publisher version (DOI)

http://dx.doi.org/10.1039/d2sc04945g