Wet spinning of hollow graphene fibers with high capacitance

Publication Name

Chemical Engineering Journal

Abstract

Herein, we report a facile coaxial wet-spinning strategy to continuously produce hollow graphene fibers (HGF) with the merits of high conductivity, excellent flexibility, and enhanced electrode–electrolyte contact. The hollow structure is achieved by introducing reductant-containing coagulant solution into the fiber core with a composition identical to the spinning bath. The produced fibers were assembled into a supercapacitor device with an ultra-high specific capacitance of 711 mF/cm2 (i.e. 33.5 mF/cm or 190F/cm3). The combination of outstanding electrochemical and mechanical properties makes this HGF a promising candidate for use in wearable supercapacitors and electronics.

Open Access Status

This publication is not available as open access

Volume

453

Article Number

139920

Funding Number

CE 140100012

Funding Sponsor

Australian National Fabrication Facility

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Link to publisher version (DOI)

http://dx.doi.org/10.1016/j.cej.2022.139920