Polyamide-6-based composites reinforced with pristine or functionalized multi-walled carbon nanotubes produced using melt extrusion technique

RIS ID

105849

Publication Details

Mahmood, N., Islam, M., Hameed, A., Saeed, S. & Khan, A. Nawaz. (2014). Polyamide-6-based composites reinforced with pristine or functionalized multi-walled carbon nanotubes produced using melt extrusion technique. Journal of Composite Materials, 48 (10), 1197-1207.

Abstract

Polyamide-6-based composites with pristine or functionalized multi-walled carbon nanotubes were produced using melt extrusion technique. After chemical functionalization, defect formation and attachment of carboxylic (−COOH) or amine (−NH2) groups on carbon nanotubes was confirmed from high-resolution transmission electron microscope and Fourier transform infra-red spectroscope studies. Carbon nanotubes incorporation promoted growth of α-form crystals with enhanced thermal stability through increase in crystallization temperature from 162 to 192℃. Dynamic mechanical thermal analysis (DMTA) indirectly pointed out to a homogeneous, uniform dispersion of nanotubes with reduction in free volume of the polymer, exhibiting a slight increase in glass transition temperature and a significant drop in coefficient of thermal expansion value. Composites containing 0.5 wt% NH2-carbon nanotubes show increases in elastic modulus and tensile strength by ∼60 and 76%, respectively. Uniform dispersion and high interfacial strength was manifested by drop in strain to failure and lack of evidence of carbon nanotubes debonding from the matrix.

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Link to publisher version (DOI)

http://dx.doi.org/10.1177/0021998313484779