Degree Name

Doctor of Philosophy


Inteligent Polymer Research Institute


Artificial muscle technology has seen vast advancements since its inception in the 1950s. The impetus for artificial muscle research is to overcome many of the inherent short comings of traditional actuators such as their limited scalability and movement flexibility. In an effort to further advance the field of artificial muscles this thesis focused on the twisted composite fibre variety of artificial muscles, and aimed to improve on the current state-of-the-art through a better understanding of the fundamental mechanics that drive these actuators, and optimisation of materials, compositions and preparation technique.

Niobium yarns containing a volume changing hydrogel guest material exhibited the ability to actuate torsionally under a certain stimulus, that is: exert a torque and generate a torsional stroke of up to 175°/mm. These torsional actuators were used to test a theoretical model for predicting torsional stroke with good correspondence between empirical and theoretical outcomes. The niobium yarns were, however, inconsistent in fabrication, which led to the desire to improve methods for fabricating twisted composite fibres. A range of material types were compared qualitatively and quantitatively using a screening method for preparation of optimised twisted fibre yarns. Notably, cotton and silk yarns performed well when used in composites with a specific hydrogel achieving ~60% unaided return up-twist post actuation. Due to its favourable performance and fibre morphology, cotton was chosen for further experiments. It was imbued with HydroMed hydrogel and showed torsional actuation through swelling-deswelling mechanisms comparable with actuators made from more exotic materials which were described in the literature.

FoR codes (2008)

030399 Macromolecular and Materials Chemistry not elsewhere classified, 091202 Composite and Hybrid Materials, 091205 Functional Materials, 091209 Polymers and Plastics



Unless otherwise indicated, the views expressed in this thesis are those of the author and do not necessarily represent the views of the University of Wollongong.